大气中一氧化碳浓度变化的模拟研究   总被引：4，自引：1，他引：4  

张仁健  王明星 《大气科学》2001,25(6):847-855

应用全球二维大气化学模式,模拟了CO、CH4和OH自由基等成分自工业革命到2020年的长期变化.模拟的全球CO平均体积分数在1840年、1991年和2020年分别为27×10-6、76×10-6和105×10-6.从1840到1991年,OH自由基数浓度从7.17×105个分子/cm3下降到5.79×105个分子/cm3,降低了19%.模拟的CH4长期变化与冰芯资料相符.模拟的20世纪80年代CO体积分数年增长率为1.03%～1.06%.大气中CO在20世纪90年代前是增长的,而到90年代初观测到CO体积分数突然下降.应用二维大气化学模式对此原因进行了模拟研究,结果表明,CO排放源的减少是CO体积分数下降的主要因子,平流层臭氧减少是另一个重要因子.尽管CO排放源的减少对大气CH4增长率的变化有较大影响,而CH4排放源减少对CO体积分数变化却几乎没有影响.  相似文献   

NUMERICAL SIMULATION OF ATMOSPHERIC METHANE TRENDS OVER THE LAST 150 YEARS     

张仁健  王明星 《Acta Meteorologica Sinica》2001,(1)

A global two-dimensional chemistry model is developed to study long-term trends of CH_4 sinceindustrial revolution.The sources of CH_4,CO and NO_x are parameterized as functions of latitudeand time.With two long-term emission scenarios,long-term trends of CH_4 are simulated.The resultshave a good agreement with observation from ice cores.The modeled CH_4 increased from 760 ppbvin 1840 to 1611.9 ppbv in 1991, while the modeled number concentration of tropospheric OHdecreased from 7.17×10~5 cm~(-3)in 1840 to 5.79×10~5 cm~(-3) in 1991.The increase of atmosphericCH_4 can be explained by the increase of emission of CH_4 and build-up because of decrease of OHradicals that remove CH_4 from the atmosphere.The model is also used to simulate the distribution of CH_4.Comparisons between the modelresults and observations show that the model can simulate both latitudinal distribution and seasonalvariation of CH_4 well.  相似文献   

NUMERICAL SIMULATION OF METHANE EMISSIONS FROM RICE PADDY FIELDS IN THE YANGTZE DELTA OF CHINA^*     

LIU Jiandong  HOU Xiuji  ZHANG Yu 《Acta Meteorologica Sinica》2001,15(1):1-11

A numerical simulation model is presented in this paper,which comprises the processes of crop growth,soil organic carbon decomposition,and methane emissions in agroecosystems.Simulation results show that the model can simulate the main process of methane emissions well,and the correlation coefficient between the simulated values and observed data is 0.79 with 239 samples,which passed a significance test of 0.01.The average error of methane emission simulation in whole growth period is about 15%.Numerical analysis of the model indicates that the average temperature during rice growth period has much impacts on methane emissions,and the basic trend of interannual methane emissions is similar to that of average temperature.The amount of methane emissions reduces about 34.93%,when the fertilizer is used instead of manure in single rice paddy.  相似文献   

NUMERICAL SIMULATION OF ATMOSPHERIC METHANE TRENDS OVER THE LAST 150 YEARS^*     

ZHANG Renjian  WANG Mingxing 《Acta Meteorologica Sinica》2001,15(1):12-20

A global two-dimensional chemistry model is developed to study long-term trends of CH₄ since industrial revolution.The sources of CH₄,CO and NO_x are parameterized as functions of latitude and time.With two long-term emission scenarios,long-term trends of CH₄ are simulated.The results have a good agreement with observation from ice cores.The modeled CH₄ increased from 760 ppbv in 1840 to 1611.9 ppbv in 1991, while the modeled number concentration of tropospheric OH decreased from 7.17×10⁵ cm^-3 in 1840 to 5.79×10⁵ cm^-3 in 1991.The increase of atmospheric CH₄ can be explained by the increase of emission of CH₄ and build-up because of decrease of OH radicals that remove CH₄ from the atmosphere.The model is also used to simulate the distribution of CH₄.Comparisons between the model results and observations show that the model can simulate both latitudinal distribution and seasonal variation of CH₄ well.  相似文献   

REMOTE SENSING OF THE SEASONAL VARIATION IN COLUMN ABUNDANCE OF ATMOSPHERIC CH₄^*          下载免费PDF全文

WEI Heli  LIU Qinghong  XU Qingshan  ZHAO Fengsheng  SONG Zhengfang 《Acta Meteorologica Sinica》2001,15(2):249-256

Infrared solar spectra on clear days were measured automatically by an infrared solar spectrometer(ISS) with 0.4 cm^-1 resolution developed by us.A line-by line(LBL) computation method was used to calculate theoretical atmospheric absorption.In the wavelength range of 3.410-3.438 μm.the absorption is mainly due to atmospheric methane and water vapor.Columnatmospheric methane was retrieved from the recorded infrared solar spectra.The seasonal variation of column atmospheric methane in Hefei has been obtained from the measuremental data of nearly 18 months since the April of 1997.and found that it is similar to that of background data.The instruments.principles of measurement and some of results were introduced,and the results are also discussed briefly in the paper.  相似文献   

我国煤层气储层研究现状及发展趋势   总被引：23，自引：0，他引：23  

蔚远江  杨起  刘大锰  黄文辉 《地质科技情报》2001,20(1):56-60

通过对煤层气储层描述及储层评价，煤储层分布，预测及选区评价，煤储层研究方法及实验技术等方面的系统评述后认为，我国目前已基本掌握了煤储层地质特征研究和地质评价选区技术，煤层气储层工程技术和储层模拟软件系统，并在煤层气储层研究方面有所突破，但我国煤储层的构造复杂，煤层多强烈变形，煤层结构常呈碎粒状及糜棱状等，煤储层多为贫煤和无烟煤，呈“三低一高”（煤层压力较低，煤层渗透率低，在水压裂等强化措施下形成的常规破裂裂缝所占比较低；煤层普遍具有较高的吸附力）的物性特征，且变质程度偏高，高煤级煤（贫煤一无烟煤）占49％，独具“中国特色”，进而讨论了当前我国煤层气储层研究急待解决的8个方面的科技问题和难点，指出了在21世纪初中我国煤层气储层研究的7个发展趋势。  相似文献   

水--煤层气两相流体在煤层中的渗流规律   总被引：1，自引：1，他引：1  

张永利  邰英楼  王来贵 《地质灾害与环境保护》2001,12(4):63-66

采用煤体承受有效应力、水-气混合流动及固一流相互作用的基本原理，建立了煤层气开采过程中水-煤层气两相流渗的基本方程，通过自行设计的实验装置，测定了煤层中水-煤层气共同流动时的两相流体的流量，渗透率及随水的饱和度变化关系，并据此模拟出了反映水-煤层气渗透基本规律，从而为煤层气开采提供了理论基础。  相似文献   

煤层煤质和含气量的测井评价方法及其应用   总被引：8，自引：0，他引：8  

董红  侯俊胜  李能根  汪浩 《物探与化探》2001,25(2):138-143

根据辽河油田东部凹陷煤储层的地质特征以及实际煤岩芯分析资料和测井资料,利用回归分析方法得出了计算煤层各组分含量和煤阶的方法;通过分析煤层气特征,利用兰氏方程、吸附等温线和煤层气层中子背景值导出了煤层含气量的计算公式,并通过辽河油田东部凹陷实际煤储层测井资料的处理解释验证了方法的有效性。  相似文献   

内蒙古兴和地区太古宙孔兹岩系变质峰期流体特征     

董永胜  周喜文 《吉林大学学报(地球科学版)》2001,31(2):122-125

为了查明麻粒岩相变质高峰期的流体特征 ,对研究区太古宙孔兹岩系变质峰期特征矿物夕线石中具负晶形的碳质液相包裹体进行了冷热台显微测温和激光拉曼光谱成分测定。研究表明 ,该类包裹体xH2 O很低 (0mol%～ 17mol% ) ,碳质成分很高 (xCO2 +CH4=70mol %～ 90mol% ) ,密度为0 .94～ 1.0g/cm3 ,相应压力约为 0 .7GPa。流体氧逸度的lg fO2 在 - 14～ - 16之间。研究结果表明 ,丰富的碳质组分不是深部来源的 ,而可能是由孔兹岩系原岩中有机质氧化作用产生。  相似文献   

煤层气产出过程中气—水两相流与煤岩变形耦合数学模型研究   总被引：1，自引：1，他引：1  

林良俊  马凤山 《水文地质工程地质》2001,28(1):1-3

气－水二相流和煤岩变形耦合作用是煤层气产出过程中一种复杂的物理现象，为准确描述这一现象，本文建立了气－水二相流和煤岩变形的微分方程，并用有限元分别将它们进行离散化，然后讨论了煤岩变形模型和气－水二相流模型进行耦合数值求解的方法。  相似文献